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Taguchi, Shigeo; Miyauchi, Hironari*; Horigome, Kazushi; Yamamoto, Masahiko; Kuno, Takehiko
Bunseki Kagaku, 67(11), p.681 - 686, 2018/11
In thermal ionization mass spectrometry, de-gassing is one of the important treatments to release impurities of filaments and to minimize the influence of background. In this work, the effect of the surface change in the tungsten filament induced by the conductively heating treatment on uranium isotopic (U/U) measurement has been investigated. It was found that the conductively heating treatment of the filament has the effect of smoothing the surface of the filament and also has the effect of improving the deposition of the sample on the filament surface. As a result of either these effects, the precision of uranium isotopic (U/U) measurement was improved.
Okubo, Ayako; Shinohara, Nobuo; Magara, Masaaki
Journal of Radioanalytical and Nuclear Chemistry, 314(1), p.231 - 234, 2017/10
Times Cited Count:2 Percentile:19.65(Chemistry, Analytical)The model date of two enriched uranium materials were determined using a new method for nuclear forensics investigation. In this method, the Th/U ratio was calculated without spike addition from measured ratios of Th/Th and U/U, and calculated Th/U ratio in secular equilibrium. The obtained model date for the low-enriched uranium material was agreed with the known production date within uncertainty. For the highly enriched uranium material, slightly younger model date than the known production date was obtained. The U interference on Th counting in thermal ionization mass spectrometry measurement was suspected as a potential cause.